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Amines - Method of Preparation of Diazonium Salts

Grade 12CBSEChemistry

Review the key concepts, formulae, and examples before starting your quiz.

🔑Concepts

Diazotization is the process of converting primary aromatic amines into diazonium salts by treating them with nitrous acid (HNO2HNO_2) at low temperatures (273278 K273\text{--}278\ K).

Nitrous acid is highly unstable and is therefore produced in situ by the reaction of sodium nitrite (NaNO2NaNO_2) with a mineral acid like HClHCl or H2SO4H_2SO_4.

The reaction must be carried out at 0C0^\circ C to 5C5^\circ C. If the temperature rises, the diazonium salt decomposes, reacting with water to form phenol and evolving N2N_2 gas.

Aromatic diazonium salts are relatively stable due to the dispersal of the positive charge over the benzene ring through resonance.

Primary aliphatic amines react with nitrous acid to form highly unstable aliphatic diazonium salts, which decompose immediately to yield a mixture of alcohols, alkenes, and alkyl halides, with the evolution of N2N_2 gas.

📐Formulae

C6H5NH2+NaNO2+2HCl273278 KC6H5N2+Cl+NaCl+2H2OC_6H_5NH_2 + NaNO_2 + 2HCl \xrightarrow{273-278\ K} C_6H_5N_2^+Cl^- + NaCl + 2H_2O

NaNO2+HClHNO2+NaClNaNO_2 + HCl \rightarrow HNO_2 + NaCl

[C6H5NN]+Cl (Benzenediazonium chloride)[C_6H_5N \equiv N]^+Cl^- \text{ (Benzenediazonium chloride)}

💡Examples

Problem 1:

Explain why aniline does not form a stable diazonium salt at room temperature.

Solution:

At room temperature (above 278 K278\ K), the benzenediazonium salt formed is thermally unstable. It reacts with the water present in the reaction mixture via a nucleophilic substitution reaction: C6H5N2+Cl+H2OC6H5OH+N2+HClC_6H_5N_2^+Cl^- + H_2O \rightarrow C_6H_5OH + N_2 + HCl.

Explanation:

The diazonium group (N2+-N_2^+) is an excellent leaving group. The kinetic energy at room temperature is sufficient to break the CNC-N bond, leading to the formation of phenol and the release of nitrogen gas.

Problem 2:

How is nitrous acid prepared during the diazotization reaction?

Solution:

Nitrous acid (HNO2HNO_2) is prepared in the reaction flask (in situ) by reacting sodium nitrite (NaNO2NaNO_2) with cold dilute hydrochloric acid (HClHCl): NaNO2+HClHNO2+NaClNaNO_2 + HCl \rightarrow HNO_2 + NaCl.

Explanation:

Since HNO2HNO_2 is an unstable weak acid that decomposes easily, it cannot be stored and must be generated freshly at the time of the reaction.

Method of Preparation of Diazonium Salts Revision - Class 12 Chemistry CBSE